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A climatology of 7Be in surface air in European Union

机译:欧盟地表空气中7Be的气候

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摘要

This study presents the first European-wide analysis of the spatial and temporal distribution of the cosmogenic isotope 7Be in surface air. The long term database of the 34 sampling sites that regularly provide data to the Radioactivity Environmental Monitoring (REM) network, managed by the Joint Research Centre (JRC) in Ispra, was used. While temporal coverage varies between stations, some of them have delivered data more or less continuously from 1984 to 2011. The station locations were considerably heterogeneous, both in terms of latitude and altitude, a range which should ensure a high degree of representativeness of the results. The mean values of 7Be activity concentration presented a spatial distribution value ranging from 2.0 to 5.4 mBq/m3 over the European Union. The results of the ANOVA analysis of all 7Be data available indicated that its temporal and spatial distributions were mainly explained by the location and characteristic of the sampling sites rather than its temporal distribution (yearly, seasonal and monthly). Higher 7Be concentrations were registered at the middle, compared to high-latitude, regions. However, there was no correlation with altitude, since all stations are sited within the atmospheric boundary layer. In addition, the total and yearly analyses of the data indicated a dynamic range of 7Be activity for each solar cycle and phase (maximum or minimum), different impact on stations having been observed according to their location. Finally, the results indicated a significant seasonal and monthly variation for 7Be activity concentration across the European Union, with maximum concentrations occurring in the summer and minimum in the winter, although with differences in the values reached. The knowledge of the horizontal and vertical distribution of this natural radionuclide in the atmosphere is a key parameter for modelling studies of atmospheric processes, which are important phenomena to be taken into account in the case of a nuclear accident.
机译:这项研究提出了第一个欧洲范围内对地表空气中宇宙成因同位素7Be的时空分布的分析。使用了由Ispra联合研究中心(JRC)管理的,定期向放射性环境监测(REM)网络提供数据的34个采样点的长期数据库。尽管各个站点的时间覆盖范围有所不同,但其中一些站点从1984年到2011年或多或少连续地提供了数据。站点的位置在纬度和海拔高度上都非常不同,该范围应确保结果的高度代表性。 7Be活度浓度的平均值在欧盟范围内的空间分布值为2.0到5.4 mBq / m3。所有7Be数据的ANOVA分析结果表明,其时间和空间分布主要是由采样地点的位置和特征来解释的,而不是其时间分布(每年,季节性和每月)。与高纬度地区相比,中部的7Be浓度更高。但是,由于所有测站都位于大气边界层内,因此与海拔高度无关。此外,对数据的总体和年度分析表明,每个太阳周期和每个相位(最大或最小)的7Be活动动态范围,已根据其位置观测到对站的不同影响。最后,结果表明整个欧盟7Be活性浓度存在明显的季节性和每月变化,最大浓度发生在夏季,冬季最小,尽管两者之间存在差异。大气中这种天然放射性核素的水平和垂直分布的知识是对大气过程进行建模研究的关键参数,这是发生核事故时要考虑的重要现象。

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